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Introducing superconductivity in topological materials can lead to innovative electronic phases and device functionalities. Here, we present a unique strategy for quantum engineering of superconducting junctions in moiré materials through direct, on-chip, and fully encapsulated 2D crystal growth. We achieve robust and designable superconductivity in Pd-metalized twisted bilayer molybdenum ditelluride (MoTe2) and observe anomalous superconducting effects in high-quality junctions across ~20 moiré cells. Unexpectedly, the junction develops enhanced, instead of weakened, superconducting behaviors, exhibiting fluctuations to a higher critical magnetic field compared to its adjacent Pd7MoTe2superconductor. In addition, the critical current further exhibits a notable V-shaped minimum at zero magnetic field. These features are unexpected in conventional Josephson junctions and absent in junctions of natural bilayer MoTe2created using the same approach. We discuss implications of these observations, including the possible formation of mixed even- and odd-parity superconductivity at the moiré junctions. Our results also demonstrate a pathway to engineer and investigate superconductivity in fractional Chern insulators.more » « lessFree, publicly-accessible full text available January 31, 2026
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Villalpando, Graciela; Jovanovic, Milena; Hoff, Brianna; Jiang, Yi; Singha, Ratnadwip; Yuan, Fang; Hu, Haoyu; Călugăru, Dumitru; Mathur, Nitish; Khoury, Jason F; et al (, Science Advances)Flat bands that do not merely arise from weak interactions can produce exotic physical properties, such as superconductivity or correlated many-body effects. The quantum metric can differentiate whether flat bands will result in correlated physics or are merely dangling bonds. A potential avenue for achieving correlated flat bands involves leveraging geometrical constraints within specific lattice structures, such as the kagome lattice; however, materials are often more complex. In these cases, quantum geometry becomes a powerful indicator of the nature of bands with small dispersions. We present a simple, soft-chemical processing route to access a flat band with an extended quantum metric below the Fermi level. By oxidizing Ni-kagome material Cs2Ni3S4to CsNi3S4, we see a two orders of magnitude drop in the room temperature resistance. However, CsNi3S4is still insulating, with no evidence of a phase transition. Using experimental data, density functional theory calculations, and symmetry analysis, our results suggest the emergence of a correlated insulating state of unknown origin.more » « less
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Pollak, Connor J; Skorupskii, Grigorii; Gutierrez-Amigo, Martin; Singha, Ratnadwip; Stiles, Joseph W; Kamm, Franziska; Pielnhofer, Florian; Ong, N P; Errea, Ion; Vergniory, Maia G; et al (, Journal of the American Chemical Society)
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